56. The Velvet Underground - "I'm Set Free" (from the self-titled album, MGM Records, 1969)
Guitar solos are sweet, but I rarely listen to songs only for the solo. The rest of this song is good too, but the solo is one of those sublime moments that elevates every moment spent in its company.
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See:
Sinister Minister's solo, "I Believe I Can Fly"
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